Coordination engineering of heterogeneous high-valent Fe(IV)-oxo for safe removal of pollutants via powerful Fenton-like reactions
Abstract Coordination engineering Room Spray of high-valent Fe(IV)-oxo (FeIV=O) is expected to break the activity-selectivity trade-off of traditional reactive oxygen species, while attempts to regulate the oxidation behaviors of heterogeneous FeIV=O remain unexplored.Here, by coordination engineering of Fe-Nx single-atom catalysts (Fe-Nx SACs), we